A comparative perspective of electrochemical and photochemical approaches for catalytic H2O2 production

dc.contributor.authorSun, Yanyan
dc.contributor.authorHan, Lei
dc.contributor.authorStrasser, Peter
dc.date.accessioned2020-08-17T08:55:53Z
dc.date.available2020-08-17T08:55:53Z
dc.date.issued2020-08-06
dc.description.abstractHydrogen peroxide (H2O2) has a wide range of important applications in various fields including chemical industry, environmental remediation, and sustainable energy conversion/storage. Nevertheless, the stark disconnect between today's huge market demand and the historical unsustainability of the currently-used industrial anthraquinone-based production process is promoting extensive research on the development of efficient, energy-saving and sustainable methods for H2O2 production. Among several sustainable strategies, H2O2 production via electrochemical and photochemical routes has shown particular appeal, because only water, O2, and solar energy/electricity are involved during the whole process. In the past few years, considerable efforts have been devoted to the development of advanced electrocatalysts and photocatalysts for efficient and scalable H2O2 production with high efficiency and stability. In this review, we compare and contrast the two distinct yet inherently closely linked catalytic processes, before we detail recent advances in the design, preparation, and applications of different H2O2 catalyst systems from the viewpoint of electrochemical and photochemical approaches. We close with a balanced perspective on remaining future scientific and technical challenges and opportunities.en
dc.description.sponsorshipBMWi, 0350013A, ChemEFlex - Umsetzbarkeitsanalyse zur Lastflexibilisierung elektrochemischer Verfahren in der Industrie; Teilvorhaben: Modellierung der Chlor-Alkali-Elektrolyse sowie anderer Prozesse und deren Bewertung hinsichtlich Wirtschaftlichkeit und möglicher Hemmnisseen
dc.description.sponsorshipEC/H2020/779366 /EU/Critical Raw material ElectrocatalystS replacement ENabling Designed pOst-2020 PEMFC/CRESCENDOen
dc.description.sponsorshipTU Berlin, Open-Access-Mittel - 2020en
dc.identifier.eissn1460-4744
dc.identifier.issn0306-0012
dc.identifier.urihttps://depositonce.tu-berlin.de/handle/11303/11572
dc.identifier.urihttp://dx.doi.org/10.14279/depositonce-10459
dc.language.isoenen
dc.rights.urihttps://creativecommons.org/licenses/by/3.0/en
dc.subject.ddc540 Chemie und zugeordnete Wissenschaftende
dc.subject.othercatalysisen
dc.subject.otherH2O2 productionen
dc.subject.otherhydrogen peroxideen
dc.subject.otherelectrochemistryen
dc.subject.otherphotochemistryen
dc.titleA comparative perspective of electrochemical and photochemical approaches for catalytic H2O2 productionen
dc.typeArticleen
dc.type.versionpublishedVersionen
dcterms.bibliographicCitation.doi10.1039/D0CS00458Hen
dcterms.bibliographicCitation.journaltitleChemical Society Reviewsen
dcterms.bibliographicCitation.originalpublishernameRoyal Society of Chemistry (RSC)en
dcterms.bibliographicCitation.originalpublisherplaceCambridgeen
tub.accessrights.dnbfreeen
tub.affiliationFak. 2 Mathematik und Naturwissenschaften::Inst. Chemie::FG Technische Chemiede
tub.affiliation.facultyFak. 2 Mathematik und Naturwissenschaftende
tub.affiliation.groupFG Technische Chemiede
tub.affiliation.instituteInst. Chemiede
tub.publisher.universityorinstitutionTechnische Universität Berlinen

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