Fe-POM/attapulgite composite materials: Efficient catalysts for plastic pyrolysis

dc.contributor.authorAttique, Saira
dc.contributor.authorBatool, Madeeha
dc.contributor.authorGoerke, Oliver
dc.contributor.authorAbbas, Ghayoor
dc.contributor.authorSaeed, Faraz Ahmad
dc.contributor.authorDin, Muhammad Imran
dc.contributor.authorJalees, Irfan
dc.contributor.authorIrfan, Ahmad
dc.contributor.authorGregory, Duncan H
dc.contributor.authorTufail Shah, Asma
dc.date.accessioned2022-09-07T09:25:30Z
dc.date.available2022-09-07T09:25:30Z
dc.date.issued2022-09-01
dc.date.updated2022-08-22T12:11:52Z
dc.descriptionDieser Beitrag ist mit Zustimmung des Rechteinhabers aufgrund einer (DFG geförderten) Allianz- bzw. Nationallizenz frei zugänglich.de
dc.descriptionThis publication is with permission of the rights owner freely accessible due to an Alliance licence and a national licence (funded by the DFG, German Research Foundation) respectively.en
dc.description.abstractThis article describes the catalytic cracking of low-density polyethylene over attapulgite clay and iron substituted tungstophosphate/attapulgite clay (Fe-POM/attapulgite) composite materials to evaluate their suitability and performance for recycling of plastic waste into liquid fuel. The prepared catalysts enhanced the yield of liquid fuel (hydrocarbons) produced in cracking process. A maximum yield of 82% liquid oil fraction with a negligible amount of coke was obtained for 50% Fe-POM/attapulgite composite. Whereas, only 68% liquid oil fractions with a large amount of solid black residue was produced in case of non-catalytic pyrolysis. Moreover, Fe-POM/attapulgite clay composites showed higher selectivity towards lower hydrocarbons (C5–C12) with aliphatic hydrocarbons as major fractions. These synthesised composite catalysts significantly lowered the pyrolysis temperature from 375°C to 310°C. Hence, recovery of valuable fuel oil from polyethylene using these synthesised catalysts suggested their applicability for energy production from plastic waste at industrial level as well as for effective environment pollution control.en
dc.identifier.eissn1096-3669
dc.identifier.issn0734-242X
dc.identifier.urihttps://depositonce.tu-berlin.de/handle/11303/17374
dc.identifier.urihttp://dx.doi.org/10.14279/depositonce-16155
dc.language.isoenen
dc.rights.urihttp://rightsstatements.org/vocab/InC/1.0/en
dc.subject.ddc690 Hausbau, Bauhandwerkde
dc.subject.otherwaste recyclingen
dc.subject.otherpyrolysisen
dc.subject.othertungstophosphateen
dc.subject.otherliquid hydrocarbonen
dc.subject.otherpolyethyleneen
dc.subject.otherGC-MSen
dc.titleFe-POM/attapulgite composite materials: Efficient catalysts for plastic pyrolysisen
dc.typeArticleen
dc.type.versionpublishedVersionen
dcterms.bibliographicCitation.doi10.1177/0734242X221080084en
dcterms.bibliographicCitation.issue9en
dcterms.bibliographicCitation.journaltitleWaste Management & Researchen
dcterms.bibliographicCitation.originalpublishernameSageen
dcterms.bibliographicCitation.originalpublisherplaceLondonen
dcterms.bibliographicCitation.pageend1439en
dcterms.bibliographicCitation.pagestart1433en
dcterms.bibliographicCitation.volume40en
tub.accessrights.dnbembargoed*
tub.affiliationFak. 3 Prozesswissenschaften::Inst. Werkstoffwissenschaften und -technologien::FG Keramische Werkstoffede
tub.affiliation.facultyFak. 3 Prozesswissenschaftende
tub.affiliation.groupFG Keramische Werkstoffede
tub.affiliation.instituteInst. Werkstoffwissenschaften und -technologiende
tub.publisher.universityorinstitutionTechnische Universität Berlinen

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