Enhanced catalytic performance of MnxOy-Na2WO4/SiO2 for the oxidative coupling of methane using an ordered mesoporous silica support

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dc.contributor.authorYildiz, M.
dc.contributor.authorAksu, Y.
dc.contributor.authorSimon, U.
dc.contributor.authorKailasam, K.
dc.contributor.authorGörke, O.
dc.contributor.authorRosowski, F.
dc.contributor.authorSchomäcker, R.
dc.contributor.authorThomas, A.
dc.contributor.authorArndt, S.
dc.date.accessioned2016-06-21T08:29:20Z
dc.date.available2016-06-21T08:29:20Z
dc.date.issued2014
dc.description.abstractThe oxidative coupling of methane is a highly promising reaction for its direct conversion. Silica supported MnxOy–Na2WO4 is a suitable catalyst for this reaction. In this study, a variety of different SiO2 materials have been tested as supports. Surprisingly, the application of ordered mesoporous silicas, here exemplarily shown for SBA-15 as support materials, greatly enhances the catalytic performance. The CH4 conversion increased two fold and also the C2 selectivity is strongly increased.en
dc.identifier.eissn1359-7345
dc.identifier.pmid25302934
dc.identifier.urihttps://depositonce.tu-berlin.de/handle/11303/5574
dc.identifier.urihttp://dx.doi.org/10.14279/depositonce-5203
dc.language.isoen
dc.rights.urihttps://creativecommons.org/licenses/by/3.0/
dc.subject.ddc540 Chemie und zugeordnete Wissenschaftende
dc.titleEnhanced catalytic performance of MnxOy-Na2WO4/SiO2 for the oxidative coupling of methane using an ordered mesoporous silica supporten
dc.typeArticleen
dc.type.versionpublishedVersionen
dcterms.bibliographicCitation.doi10.1039/c4cc06561a
dcterms.bibliographicCitation.issue92
dcterms.bibliographicCitation.journaltitleChemical communicationsen
dcterms.bibliographicCitation.originalpublishernameRoyal Society of Chemistryde
dcterms.bibliographicCitation.originalpublisherplaceCambridgede
dcterms.bibliographicCitation.pageend14442
dcterms.bibliographicCitation.pagestart14440
dcterms.bibliographicCitation.volume50
tub.accessrights.dnbfree
tub.affiliationVerbundforschung::Exzellenzcluster (EXC)::EXC - UniCatde
tub.affiliationFak. 3 Prozesswissenschaften::Inst. Werkstoffwissenschaften und -technologien::FG Keramische Werkstoffede
tub.affiliation.facultyVerbundforschungde
tub.affiliation.facultyFak. 3 Prozesswissenschaftende
tub.affiliation.groupEXC - UniCatde
tub.affiliation.groupFG Keramische Werkstoffede
tub.affiliation.instituteExzellenzcluster (EXC)de
tub.affiliation.instituteInst. Werkstoffwissenschaften und -technologiende
tub.publisher.universityorinstitutionTechnische Universität Berlin

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