Higher alcohol synthesis over Rh catalysts: conditioning of Rh/N-CNTs by Co and Mn entrapped in the support
| dc.contributor.author | Xie, Zailai | |
| dc.contributor.author | Frank, Benjamin | |
| dc.contributor.author | Huang, Xing | |
| dc.contributor.author | Schlögl, Robert | |
| dc.contributor.author | Trunschke, Annette | |
| dc.date.accessioned | 2018-05-25T11:08:04Z | |
| dc.date.available | 2018-05-25T11:08:04Z | |
| dc.date.issued | 2016-10-13 | |
| dc.description.abstract | Rh nanoparticles supported on commercial non-purified N-doped CNTs (NCNTs) containing residual CNT growth catalyst have been studied in hydrogenation of CO to higher alcohols. It has been found that Co and Mn residues in NCNTs are not inert, but change the catalyst under reaction conditions and efficiently promote the catalyst resulting in both increasing activity and selectivity to C2+ alcohols with time on stream. | en |
| dc.description.sponsorship | BMBF, 03X0204C, CarboKat - Einsatz von Carbon Nanotubes als Katalysator und Katalysatorträger | en |
| dc.identifier.eissn | 1572-879X | |
| dc.identifier.issn | 1011-372X | |
| dc.identifier.uri | https://depositonce.tu-berlin.de/handle/11303/7846 | |
| dc.identifier.uri | http://dx.doi.org/10.14279/depositonce-7006 | |
| dc.language.iso | en | en |
| dc.rights.uri | https://creativecommons.org/licenses/by/4.0/ | en |
| dc.subject.ddc | 540 Chemie und zugeordnete Wissenschaften | de |
| dc.subject.ddc | 660 Chemische Verfahrenstechnik | de |
| dc.subject.other | Rhodium | en |
| dc.subject.other | Cobalt | en |
| dc.subject.other | Manganese | en |
| dc.subject.other | CNT growth catalyst | en |
| dc.subject.other | higher alcohol synthesis | en |
| dc.subject.other | carbon nanotubes | en |
| dc.subject.other | nitrogen doping | en |
| dc.subject.other | nanoparticles | en |
| dc.title | Higher alcohol synthesis over Rh catalysts: conditioning of Rh/N-CNTs by Co and Mn entrapped in the support | en |
| dc.type | Article | en |
| dc.type.version | publishedVersion | en |
| dcterms.bibliographicCitation.doi | 10.1007/s10562-016-1875-6 | en |
| dcterms.bibliographicCitation.issue | 12 | en |
| dcterms.bibliographicCitation.journaltitle | Catalysis Letters | en |
| dcterms.bibliographicCitation.originalpublishername | Springer Science+Business Media | en |
| dcterms.bibliographicCitation.originalpublisherplace | Dordrecht | en |
| dcterms.bibliographicCitation.pageend | 2424 | en |
| dcterms.bibliographicCitation.pagestart | 2417 | en |
| dcterms.bibliographicCitation.volume | 146 | en |
| tub.accessrights.dnb | free | en |
| tub.affiliation | Fak. 2 Mathematik und Naturwissenschaften::Inst. Chemie::FG Metallorganische Chemie und Anorganische Materialien | de |
| tub.affiliation.faculty | Fak. 2 Mathematik und Naturwissenschaften | de |
| tub.affiliation.group | FG Metallorganische Chemie und Anorganische Materialien | de |
| tub.affiliation.institute | Inst. Chemie | de |
| tub.publisher.universityorinstitution | Technische Universität Berlin | en |