Imaging molecular structure through femtosecond photoelectron diffraction on aligned and oriented gas-phase molecules

dc.contributor.authorBoll, Rebecca
dc.contributor.authorRouzée, Arnaud
dc.contributor.authorAdolph, Marcus
dc.contributor.authorAnielski, Denis
dc.contributor.authorAquila, Andrew
dc.contributor.authorBari, Sadia
dc.contributor.authorBomme, Cédric
dc.contributor.authorBostedt, Christoph
dc.contributor.authorBozek, John D.
dc.contributor.authorChapman, Henry N.
dc.contributor.authorChristensen, Lauge
dc.contributor.authorCoffee, Ryan
dc.contributor.authorCoppola, Niccola
dc.contributor.authorDe, Sankar
dc.contributor.authorDecleva, Piero
dc.contributor.authorEpp, Sascha W.
dc.contributor.authorErk, Benjamin
dc.contributor.authorFilsinger, Frank
dc.contributor.authorFoucar, Lutz
dc.contributor.authorGorkhover, Tais
dc.contributor.authorGumprecht, Lars
dc.contributor.authorHömke, André
dc.contributor.authorHolmegaard, Lotte
dc.contributor.authorJohnsson, Per
dc.contributor.authorKienitz, Jens S.
dc.contributor.authorKierspel, Thomas
dc.contributor.authorKrasniqi, Faton
dc.contributor.authorKühnel, Kai-Uwe
dc.contributor.authorMaurer, Jochen
dc.contributor.authorMesserschmidt, Marc
dc.contributor.authorMoshammer, Robert
dc.contributor.authorMueller, Nele L. M.
dc.contributor.authorRudek, Benedikt
dc.contributor.authorSavelyev, Evgeny
dc.contributor.authorSchlichting, Ilme
dc.contributor.authorSchmidt, Carlo
dc.contributor.authorScholz, Frank
dc.contributor.authorSchorb, Sebastian
dc.contributor.authorSchulz, Joachim
dc.contributor.authorSeltmann, Jörn
dc.contributor.authorStener, Mauro
dc.contributor.authorStern, Stephan
dc.contributor.authorTechert, Simone
dc.contributor.authorThøgersen, Jan
dc.contributor.authorTrippel, Sebastian
dc.contributor.authorViefhaus, Jens
dc.contributor.authorVrakking, Marc
dc.contributor.authorStapelfeldt, Henrik
dc.contributor.authorKuepper, Jochen
dc.contributor.authorUllrich, Joachim
dc.contributor.authorRudenko, Artem
dc.contributor.authorRolles, Daniel
dc.date.accessioned2016-06-21T08:29:19Z
dc.date.available2016-06-21T08:29:19Z
dc.date.issued2014
dc.description.abstractThis paper gives an account of our progress towards performing femtosecond time-resolved photoelectron diffraction on gas-phase molecules in a pump–probe setup combining optical lasers and an X-ray free-electron laser. We present results of two experiments aimed at measuring photoelectron angular distributions of laser-aligned 1-ethynyl-4-fluorobenzene (C8H5F) and dissociating, laser-aligned 1,4-dibromobenzene (C6H4Br2) molecules and discuss them in the larger context of photoelectron diffraction on gas-phase molecules. We also show how the strong nanosecond laser pulse used for adiabatically laser-aligning the molecules influences the measured electron and ion spectra and angular distributions, and discuss how this may affect the outcome of future time-resolved photoelectron diffraction experiments.en
dc.identifier.eissn1364-5498
dc.identifier.issn1359-6640
dc.identifier.pmid25290160
dc.identifier.urihttps://depositonce.tu-berlin.de/handle/11303/5570
dc.identifier.urihttp://dx.doi.org/10.14279/depositonce-5199
dc.language.isoen
dc.rights.urihttps://creativecommons.org/licenses/by/3.0/
dc.subject.ddc540 Chemie und zugeordnete Wissenschaftende
dc.titleImaging molecular structure through femtosecond photoelectron diffraction on aligned and oriented gas-phase moleculesen
dc.typeArticleen
dc.type.versionpublishedVersionen
dcterms.bibliographicCitation.doi10.1039/c4fd00037d
dcterms.bibliographicCitation.journaltitleFaraday discussionsen
dcterms.bibliographicCitation.originalpublishernameRoyal Society of Chemistryde
dcterms.bibliographicCitation.originalpublisherplaceCambridgede
dcterms.bibliographicCitation.pageend80
dcterms.bibliographicCitation.pagestart57
dcterms.bibliographicCitation.volume171
tub.accessrights.dnbfree
tub.affiliationFak. 2 Mathematik und Naturwissenschaften::Inst. Optik und Atomare Physikde
tub.affiliation.facultyFak. 2 Mathematik und Naturwissenschaftende
tub.affiliation.instituteInst. Optik und Atomare Physikde
tub.publisher.universityorinstitutionTechnische Universität Berlin

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