Future challenges in heterogeneous catalysis: understanding catalysts under dynamic reaction conditions

dc.contributor.authorKalz, Kai F.
dc.contributor.authorKrähnert, Ralph
dc.contributor.authorDvoyashkin, Muslim
dc.contributor.authorDittmeyer, Roland
dc.contributor.authorGläser, Roger
dc.contributor.authorKrewer, Ulrike
dc.contributor.authorReuter, Karsten
dc.contributor.authorGrunwaldt, Jan-Dierk
dc.date.accessioned2017-07-14T10:50:10Z
dc.date.available2017-07-14T10:50:10Z
dc.date.issued2017
dc.description.abstractIn the future, (electro-) chemical catalysts will have to be more tolerant towards a varying supply of energy and raw materials. This is mainly due to the fluctuating nature of renewable ener-gies. For example, power-to-chemical processes require a shift from steady-state operation towards operation under dynamic reaction conditions. This brings along a number of demands for the design of both catalysts and reactors, because it is well-known that the structure of catalysts is very dynamic. However, in-depth studies of catalysts and catalytic reactors under such transient conditions have only started recently. This requires studies and advances in the fields of 1) operando spectroscopy including time-resolved methods, 2) theory with predictive quality, 3) kinetic modelling, 4) design of catalysts by appropriate preparation concepts, and 5) novel/modular reactor designs. An intensive exchange between these scientific disciplines will enable a substantial gain of fundamental knowledge which is urgently required. This concept article highlights recent developments, challenges, and future directions for understanding catalysts under dynamic reaction conditions.en
dc.description.sponsorshipDFG, GR 3987/2-1en
dc.identifier.eissn1867-3899
dc.identifier.issn1867-3880
dc.identifier.pmid28239429
dc.identifier.urihttps://depositonce.tu-berlin.de/handle/11303/6486
dc.identifier.urihttp://dx.doi.org/10.14279/depositonce-5994
dc.language.isoen
dc.rights.urihttps://creativecommons.org/licenses/by-nc/4.0/
dc.subject.ddc540 Chemie und zugeordnete Wissenschaftende
dc.subject.otherelectrocatalysisen
dc.subject.otherenergy storageen
dc.subject.otherheterogeneous catalysisen
dc.subject.othermolecular modellingen
dc.subject.otheroperando spectroscopyen
dc.titleFuture challenges in heterogeneous catalysis: understanding catalysts under dynamic reaction conditionsen
dc.typeArticleen
dc.type.versionpublishedVersionen
dcterms.bibliographicCitation.doi10.1002/cctc.201600996
dcterms.bibliographicCitation.issue1
dcterms.bibliographicCitation.journaltitleChemCatChemen
dcterms.bibliographicCitation.originalpublishernameWiley-VCHen
dcterms.bibliographicCitation.originalpublisherplaceWeinheimen
dcterms.bibliographicCitation.pageend29
dcterms.bibliographicCitation.pagestart17
dcterms.bibliographicCitation.volume9
tub.accessrights.dnbfree
tub.affiliationFak. 2 Mathematik und Naturwissenschaften::Inst. Chemie::FG Technische Chemiede
tub.affiliation.facultyFak. 2 Mathematik und Naturwissenschaftende
tub.affiliation.groupFG Technische Chemiede
tub.affiliation.instituteInst. Chemiede
tub.publisher.universityorinstitutionTechnische Universität Berlin

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