Nickel as a co-catalyst for photocatalytic hydrogen evolution on graphitic-carbon nitride (sg-CN): what is the nature of the active species?

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dc.contributor.authorIndra, Arindam
dc.contributor.authorMenezes, Prashanth W.
dc.contributor.authorKailasam, Kamalakannan
dc.contributor.authorHollmann, Dirk
dc.contributor.authorSchröder, Marc
dc.contributor.authorThomas, Arne
dc.contributor.authorBrückner, Angelika
dc.contributor.authorDrieß, Matthias
dc.date.accessioned2017-10-24T07:23:06Z
dc.date.available2017-10-24T07:23:06Z
dc.date.issued2016
dc.descriptionDieser Beitrag ist mit Zustimmung des Rechteinhabers aufgrund einer (DFG geförderten) Allianz- bzw. Nationallizenz frei zugänglich.de
dc.descriptionThis publication is with permission of the rights owner freely accessible due to an Alliance licence and a national licence (funded by the DFG, German Research Foundation) respectively.en
dc.description.abstractThe nature of a nickel-based co-catalyst deposited on a sol-gel prepared porous graphitic-carbon nitride (sg-CN), for photocatalytic H-2 production from water, has been investigated. The formation of the active catalytic species, charge separation and recombination of the photogenerated electrons and holes during photochemical H-2 evolution has been determined for the first time using in situ EPR spectroscopy.en
dc.description.sponsorshipDFG, EXC 314, Unifying Concepts in Catalysisen
dc.description.sponsorshipBMBF, 03IS2071D, Light2Hydrogenen
dc.identifier.eissn1364-548X
dc.identifier.issn1359-7345
dc.identifier.pmid26498497
dc.identifier.urihttps://depositonce.tu-berlin.de/handle/11303/6914
dc.identifier.urihttp://dx.doi.org/10.14279/depositonce-6253
dc.language.isoen
dc.rights.urihttp://rightsstatements.org/vocab/InC/1.0/
dc.subject.ddc540 Chemie und zugeordnete Wissenschaftende
dc.titleNickel as a co-catalyst for photocatalytic hydrogen evolution on graphitic-carbon nitride (sg-CN): what is the nature of the active species?en
dc.typeArticleen
dc.type.versionpublishedVersionen
dcterms.bibliographicCitation.doi10.1039/c5cc07936e
dcterms.bibliographicCitation.issue1
dcterms.bibliographicCitation.journaltitleChemical communicationsen
dcterms.bibliographicCitation.originalpublishernameRoyal Society of Chemistryde
dcterms.bibliographicCitation.originalpublisherplaceCambridgede
dcterms.bibliographicCitation.pageend107
dcterms.bibliographicCitation.pagestart104
dcterms.bibliographicCitation.volume52
tub.accessrights.dnbdomain
tub.affiliationFak. 2 Mathematik und Naturwissenschaften::Inst. Chemie::FG Funktionsmaterialiende
tub.affiliationFak. 2 Mathematik und Naturwissenschaften::Inst. Chemie::FG Metallorganische Chemie und Anorganische Materialiende
tub.affiliation.facultyFak. 2 Mathematik und Naturwissenschaftende
tub.affiliation.facultyFak. 2 Mathematik und Naturwissenschaftende
tub.affiliation.groupFG Funktionsmaterialiende
tub.affiliation.groupFG Metallorganische Chemie und Anorganische Materialiende
tub.affiliation.instituteInst. Chemiede
tub.affiliation.instituteInst. Chemiede
tub.publisher.universityorinstitutionTechnische Universität Berlin

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